Facile synthesis of accordion-like porous carbon from waste PET bottles-based MIL-53(Al) and its application for high-performance Zn-ion capacitor

Uproszczony widok
dc.contributor.authorLi, Jiaxin
dc.contributor.authorZhang, Shuai
dc.contributor.authorHua, Yumeng
dc.contributor.authorLin, Yichao
dc.contributor.authorWen, Xin
dc.contributor.authorMijowska, Ewa
dc.contributor.authorTang, Tao
dc.contributor.authorChen, Xuecheng
dc.contributor.authorRuoff, Rodney
dc.contributor.organizationFaculty of Chemical Technology and Engineering, West Pomeranian University of Technology, Piastów Ave. 42, 71-065, Szczecin, Polanden
dc.contributor.organizationKey State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, 130022, Chinaen
dc.contributor.organizationSchool of Safety Engineering, China University of Mining and Technology, Xuzhou, 221116, Chinaen
dc.contributor.organizationInstitute of Advanced Electrical Materials, Qingdao University of Science and Technology, Qingdao, 266042, Chinaen
dc.contributor.organizationInstitute for Basic Science Center for Multiple Dimensional Carbon Materials, Ulsan, 44919, Republic of Koreaen
dc.contributor.organizationDepartment of Chemistry, Ulsan National Institute of Science and Technology (UNIST), Ulsan, 44919, Republic of Koreaen
dc.contributor.organizationDepartment of Materials Science and Engineering, Ulsan National Institute of Science and Technology (UNIST), Ulsan, 44919, Republic of Koreaen
dc.contributor.organizationSchool of Energy and Chemical Engineering, Ulsan National Institute of Science and Technology (UNIST), Ulsan, 44919, Republic of Koreaen
dc.contributor.organizationZachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydział Technologii i Inżynierii Chemicznejpl_PL
dc.date.accessioned2023-10-23T10:22:25Z
dc.date.available2023-10-23T10:22:25Z
dc.date.issued2023
dc.description.abstractIt is of great scientific and economic value to recycle waste poly (ethylene terephthalate) (PET) into high-value PET-based metal organic frameworks (MOFs) and further convert it into porous carbon for green energy storage applications. In the present study, a facile and cost-effective hydrothermal process was developed to direct recycle waste PET bottles into MIL-53(Al) with a 100% conversation, then the MOF-derived porous carbon was assembled into electrodes for high-performance supercapacitors. The results indicated that the as-synthesized carbon exhibited high SSA of 1712 m2 g−1 and unique accordion-like structure with hierarchical porosity. Benefit to these advantageous characters, the assembled three-electrode supercapacitor displayed high specific capacitances of 391 F g−1 at the current density of 0.5 A g−1 and good rate capability of 73.6% capacitance retention at 20 A g−1 in 6M KOH electrolyte. Furthermore, the assembled zinc ion capacitor still revealed outstanding capacitance of 335 F g−1 at 0.1 A g−1, excellent cycling stability of 92.2% capacitance retention after 10 000 cycles and ultra-high energy density of 150.3 Wh kg−1 at power density of 90 W kg−1 in 3M ZnSO4 electrolyte. It is believed that the current work provides a facile and effective strategy to recycle PET waste into high-valuable MOF, and further expands the applications of MOF-derived carbons for high-performance energy storage devices, so it is conducive to both pollution alleviation and sustainable economic development.en
dc.description.sponsorshipNational Science Centre (NCN), UMO-2020/39/B/ST8/02937en
dc.identifier.citationLi, J., Zhang, S., Hua, Y., Lin, Y., Wen, X., Mijowska, E., Tang, T., Chen, X., Ruoff, R. (2023). Facile synthesis of accordion-like porous carbon from waste PET bottles-based MIL-53(Al) and its application for high-performance Zn-ion capacitor. Green Energy & Environment. doi: 10.1016/j.gee.2023.01.002.en
dc.identifier.doihttps://doi.org/10.1016/j.gee.2023.01.002
dc.identifier.urihttps://hdl.handle.net/20.500.12539/1860
dc.language.isoenpl_PL
dc.publisherKeAi Chinese Roots Global Impacten
dc.rightsUznanie autorstwa-Użycie niekomercyjne-Bez utworów zależnych 3.0 Polska*
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/3.0/pl/*
dc.subjectPETen
dc.subjectRecyclingen
dc.subjectPorous carbonen
dc.subjectSupercapacitoren
dc.subjectEnergy storageen
dc.subject.otherDyscyplina::Nauki inżynieryjno-technicznepl_PL
dc.titleFacile synthesis of accordion-like porous carbon from waste PET bottles-based MIL-53(Al) and its application for high-performance Zn-ion capacitoren
dc.typeArticleen

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